One-step synthesis of a ZIF-8/90-based type I porous liquid

Jingqiu Hu; Zhaofang Liu; Shuangyin Tang; Meng Yao; Dezhen Zhang; Mifen Cui; Dong Yang; Jihai Tang; Xu Qiao; Zhuxiu Zhang

doi:10.1039/d3dt02423g

One-step synthesis of a ZIF-8/90-based type I porous liquid

Jingqiu Hu, Zhaofang Liu, Shuangyin Tang, Meng Yao, Dezhen Zhang, Mifen Cui, Dong Yang, Jihai Tang, Xu Qiao, Zhuxiu Zhang

College of Chemical Engineering

Research output: Contribution to journal › Article › peer-review

3 Scopus citations

Abstract

A Type I porous liquid based on the mixed-linker zeolitic imidazolate framework, ZIF-8/90-PL, has been prepared by a one-step imine condensation reaction and characterized by X-ray diffraction, FT-IR spectroscopy, TGA and rheology analysis. This facile preparation strategy of a porous liquid has enormous industrial production and application potential, with over one kilogram of ZIF-8/90-PL being successfully prepared. ZIF-8/90-PL can be directly used as a liquid absorbent or be co-processed with alumina hollow fibers to form a composite membrane with improved selectivity in the context of CO₂ separation from CH₄ or N₂. This simple synthesis method is expected to be extended to other metal-organic frameworks.

Original language	English
Pages (from-to)	17213-17218
Number of pages	6
Journal	Dalton Transactions
Volume	52
Issue number	46
DOIs	https://doi.org/10.1039/d3dt02423g
State	Published - 31 Oct 2023

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title = "One-step synthesis of a ZIF-8/90-based type I porous liquid",

abstract = "A Type I porous liquid based on the mixed-linker zeolitic imidazolate framework, ZIF-8/90-PL, has been prepared by a one-step imine condensation reaction and characterized by X-ray diffraction, FT-IR spectroscopy, TGA and rheology analysis. This facile preparation strategy of a porous liquid has enormous industrial production and application potential, with over one kilogram of ZIF-8/90-PL being successfully prepared. ZIF-8/90-PL can be directly used as a liquid absorbent or be co-processed with alumina hollow fibers to form a composite membrane with improved selectivity in the context of CO2 separation from CH4 or N2. This simple synthesis method is expected to be extended to other metal-organic frameworks.",

author = "Jingqiu Hu and Zhaofang Liu and Shuangyin Tang and Meng Yao and Dezhen Zhang and Mifen Cui and Dong Yang and Jihai Tang and Xu Qiao and Zhuxiu Zhang",

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T1 - One-step synthesis of a ZIF-8/90-based type I porous liquid

AU - Hu, Jingqiu

AU - Liu, Zhaofang

AU - Tang, Shuangyin

AU - Yao, Meng

AU - Zhang, Dezhen

AU - Cui, Mifen

AU - Yang, Dong

AU - Tang, Jihai

AU - Qiao, Xu

AU - Zhang, Zhuxiu

PY - 2023/10/31

Y1 - 2023/10/31

N2 - A Type I porous liquid based on the mixed-linker zeolitic imidazolate framework, ZIF-8/90-PL, has been prepared by a one-step imine condensation reaction and characterized by X-ray diffraction, FT-IR spectroscopy, TGA and rheology analysis. This facile preparation strategy of a porous liquid has enormous industrial production and application potential, with over one kilogram of ZIF-8/90-PL being successfully prepared. ZIF-8/90-PL can be directly used as a liquid absorbent or be co-processed with alumina hollow fibers to form a composite membrane with improved selectivity in the context of CO2 separation from CH4 or N2. This simple synthesis method is expected to be extended to other metal-organic frameworks.

AB - A Type I porous liquid based on the mixed-linker zeolitic imidazolate framework, ZIF-8/90-PL, has been prepared by a one-step imine condensation reaction and characterized by X-ray diffraction, FT-IR spectroscopy, TGA and rheology analysis. This facile preparation strategy of a porous liquid has enormous industrial production and application potential, with over one kilogram of ZIF-8/90-PL being successfully prepared. ZIF-8/90-PL can be directly used as a liquid absorbent or be co-processed with alumina hollow fibers to form a composite membrane with improved selectivity in the context of CO2 separation from CH4 or N2. This simple synthesis method is expected to be extended to other metal-organic frameworks.

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U2 - 10.1039/d3dt02423g

DO - 10.1039/d3dt02423g

M3 - 文章

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AN - SCOPUS:85176742751

SN - 1477-9226

VL - 52

SP - 17213

EP - 17218

JO - Dalton Transactions

JF - Dalton Transactions

IS - 46

ER -

One-step synthesis of a ZIF-8/90-based type I porous liquid

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