Pulsed Gas–liquid Discharge Synergistic CuFe2O4 Stimulated Fenton Reaction for Tetracycline Degradation

Pengju Chen; Yuankun Ye; Sen Wang; Zhi Fang

doi:10.1007/978-981-97-2245-7_26

Pulsed Gas–liquid Discharge Synergistic CuFe₂O₄ Stimulated Fenton Reaction for Tetracycline Degradation

Pengju Chen, Yuankun Ye, Sen Wang, Zhi Fang

COLLEGE OF ELECTRICAL ENGINEERING AND CONTROL SCIENCE

Nanjing Tech University

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Abstract

Excessive used antibiotics in various industries has caused significant impacts on both the human health and ecological environment. Low-temperature plasma, has gradually gained attentions in wastewater treatment. To improve the degradation performance of antibiotics in water, plasma coupled with catalysts are usually conducted. In this study, pulsed gas–liquid discharge coupled with CuFe₂O₄ was utilized for the degradation of tetracycline in water. The results showed that CuFe₂O₄ dosage, pulse voltage, initial concentration of tetracycline, and working gas had important effects on the degradation of tetracycline. Compared to plasma treatment alone, the plasma-catalytic system had a significant enhancement in the degradation rate. The catalytic mechanism of gas–liquid discharge synergistic CuFe₂O₄ is proposed. Radical quenching experiments showed that H₂O₂ is one of the most key active species in the plasma/CuFe₂O₄ degradation. The results of the study provide an effective way to treat antibiotics in water.

Original language	English
Title of host publication	Proceedings of the 5th International Symposium on Plasma and Energy Conversion - iSPEC 2023
Editors	Zhi Fang, Danhua Mei, Cheng Zhang, Shuai Zhang
Publisher	Springer Science and Business Media Deutschland GmbH
Pages	315-327
Number of pages	13
ISBN (Print)	9789819722440
DOIs	https://doi.org/10.1007/978-981-97-2245-7_26
State	Published - 2024
Event	5th International Symposium on Plasma and Energy Conversion, iSPEC 2023 - Nanjing, China Duration: 27 Oct 2023 → 29 Oct 2023

Publication series

Name	Springer Proceedings in Physics
Volume	398 SPP
ISSN (Print)	0930-8989
ISSN (Electronic)	1867-4941

Conference

Conference	5th International Symposium on Plasma and Energy Conversion, iSPEC 2023
Country/Territory	China
City	Nanjing
Period	27/10/23 → 29/10/23

Keywords

Fenton reaction
Gas–liquid discharge
Synergistic effect
Tetracycline degradation

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1007/978-981-97-2245-7_26

Cite this

Chen, P., Ye, Y., Wang, S., & Fang, Z. (2024). Pulsed Gas–liquid Discharge Synergistic CuFe₂O₄ Stimulated Fenton Reaction for Tetracycline Degradation. In Z. Fang, D. Mei, C. Zhang, & S. Zhang (Eds.), Proceedings of the 5th International Symposium on Plasma and Energy Conversion - iSPEC 2023 (pp. 315-327). (Springer Proceedings in Physics; Vol. 398 SPP). Springer Science and Business Media Deutschland GmbH. https://doi.org/10.1007/978-981-97-2245-7_26

Chen, Pengju ; Ye, Yuankun ; Wang, Sen et al. / Pulsed Gas–liquid Discharge Synergistic CuFe₂O₄ Stimulated Fenton Reaction for Tetracycline Degradation. Proceedings of the 5th International Symposium on Plasma and Energy Conversion - iSPEC 2023. editor / Zhi Fang ; Danhua Mei ; Cheng Zhang ; Shuai Zhang. Springer Science and Business Media Deutschland GmbH, 2024. pp. 315-327 (Springer Proceedings in Physics).

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title = "Pulsed Gas–liquid Discharge Synergistic CuFe2O4 Stimulated Fenton Reaction for Tetracycline Degradation",

abstract = "Excessive used antibiotics in various industries has caused significant impacts on both the human health and ecological environment. Low-temperature plasma, has gradually gained attentions in wastewater treatment. To improve the degradation performance of antibiotics in water, plasma coupled with catalysts are usually conducted. In this study, pulsed gas–liquid discharge coupled with CuFe2O4 was utilized for the degradation of tetracycline in water. The results showed that CuFe2O4 dosage, pulse voltage, initial concentration of tetracycline, and working gas had important effects on the degradation of tetracycline. Compared to plasma treatment alone, the plasma-catalytic system had a significant enhancement in the degradation rate. The catalytic mechanism of gas–liquid discharge synergistic CuFe2O4 is proposed. Radical quenching experiments showed that H2O2 is one of the most key active species in the plasma/CuFe2O4 degradation. The results of the study provide an effective way to treat antibiotics in water.",

keywords = "Fenton reaction, Gas–liquid discharge, Synergistic effect, Tetracycline degradation",

author = "Pengju Chen and Yuankun Ye and Sen Wang and Zhi Fang",

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Chen, P, Ye, Y, Wang, S & Fang, Z 2024, Pulsed Gas–liquid Discharge Synergistic CuFe₂O₄ Stimulated Fenton Reaction for Tetracycline Degradation. in Z Fang, D Mei, C Zhang & S Zhang (eds), Proceedings of the 5th International Symposium on Plasma and Energy Conversion - iSPEC 2023. Springer Proceedings in Physics, vol. 398 SPP, Springer Science and Business Media Deutschland GmbH, pp. 315-327, 5th International Symposium on Plasma and Energy Conversion, iSPEC 2023, Nanjing, China, 27/10/23. https://doi.org/10.1007/978-981-97-2245-7_26

Pulsed Gas–liquid Discharge Synergistic CuFe₂O₄ Stimulated Fenton Reaction for Tetracycline Degradation. / Chen, Pengju; Ye, Yuankun; Wang, Sen et al.
Proceedings of the 5th International Symposium on Plasma and Energy Conversion - iSPEC 2023. ed. / Zhi Fang; Danhua Mei; Cheng Zhang; Shuai Zhang. Springer Science and Business Media Deutschland GmbH, 2024. p. 315-327 (Springer Proceedings in Physics; Vol. 398 SPP).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

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AU - Chen, Pengju

AU - Ye, Yuankun

AU - Wang, Sen

AU - Fang, Zhi

N1 - Publisher Copyright: © The Author(s), under exclusive license to Springer Nature Singapore Pte Ltd. 2024.

PY - 2024

Y1 - 2024

N2 - Excessive used antibiotics in various industries has caused significant impacts on both the human health and ecological environment. Low-temperature plasma, has gradually gained attentions in wastewater treatment. To improve the degradation performance of antibiotics in water, plasma coupled with catalysts are usually conducted. In this study, pulsed gas–liquid discharge coupled with CuFe2O4 was utilized for the degradation of tetracycline in water. The results showed that CuFe2O4 dosage, pulse voltage, initial concentration of tetracycline, and working gas had important effects on the degradation of tetracycline. Compared to plasma treatment alone, the plasma-catalytic system had a significant enhancement in the degradation rate. The catalytic mechanism of gas–liquid discharge synergistic CuFe2O4 is proposed. Radical quenching experiments showed that H2O2 is one of the most key active species in the plasma/CuFe2O4 degradation. The results of the study provide an effective way to treat antibiotics in water.

AB - Excessive used antibiotics in various industries has caused significant impacts on both the human health and ecological environment. Low-temperature plasma, has gradually gained attentions in wastewater treatment. To improve the degradation performance of antibiotics in water, plasma coupled with catalysts are usually conducted. In this study, pulsed gas–liquid discharge coupled with CuFe2O4 was utilized for the degradation of tetracycline in water. The results showed that CuFe2O4 dosage, pulse voltage, initial concentration of tetracycline, and working gas had important effects on the degradation of tetracycline. Compared to plasma treatment alone, the plasma-catalytic system had a significant enhancement in the degradation rate. The catalytic mechanism of gas–liquid discharge synergistic CuFe2O4 is proposed. Radical quenching experiments showed that H2O2 is one of the most key active species in the plasma/CuFe2O4 degradation. The results of the study provide an effective way to treat antibiotics in water.

KW - Fenton reaction

KW - Gas–liquid discharge

KW - Synergistic effect

KW - Tetracycline degradation

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A2 - Zhang, Cheng

A2 - Zhang, Shuai

PB - Springer Science and Business Media Deutschland GmbH

T2 - 5th International Symposium on Plasma and Energy Conversion, iSPEC 2023

Y2 - 27 October 2023 through 29 October 2023

ER -

Chen P, Ye Y, Wang S, Fang Z. Pulsed Gas–liquid Discharge Synergistic CuFe₂O₄ Stimulated Fenton Reaction for Tetracycline Degradation. In Fang Z, Mei D, Zhang C, Zhang S, editors, Proceedings of the 5th International Symposium on Plasma and Energy Conversion - iSPEC 2023. Springer Science and Business Media Deutschland GmbH. 2024. p. 315-327. (Springer Proceedings in Physics). doi: 10.1007/978-981-97-2245-7_26