Syngas Production Using an Oxygen-Permeating Membrane Reactor with Cofeed of Methane and Carbon Dioxide

Zong Ping Shao; Hui Dong; Guo Xing Xiong; Wei Shen Yang

Syngas Production Using an Oxygen-Permeating Membrane Reactor with Cofeed of Methane and Carbon Dioxide

Zong Ping Shao, Hui Dong, Guo Xing Xiong, Wei Shen Yang

CAS - Dalian Institute of Chemical Physics

Research output: Contribution to journal › Article › peer-review

4 Scopus citations

Abstract

CH₄-CO₂-O₂ reforming to syngas in a novel Ba_0.5Sr_0.5Co_0.8Fe_0.2O _3-δ oxygen-permeable membrane reactor using LiLaNiO/γ-Al₂O₃ as catalyst was successfully reported. Excellent reaction performance was achieved with around 92% methane conversion efficiency, 95% CO₂ conversion rate, and nearly 8.5mL/min.cm² oxygen permeation flux. In contrast to the oxygen permeation model with the presence of large concentration of CO₂ (under such condition the oxygen permeation flux deteriorates with time), the oxygen permeation flux is really stable under the CH₄-CO₂-O₂ reforming condition.

Original language	English
Pages (from-to)	631-634
Number of pages	4
Journal	Chinese Chemical Letters
Volume	11
Issue number	7
State	Published - Jul 2000
Externally published	Yes

Keywords

Ceramic membrane reactor
Methane
Oxygen permeation
Syngas

Cite this

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title = "Syngas Production Using an Oxygen-Permeating Membrane Reactor with Cofeed of Methane and Carbon Dioxide",

abstract = "CH4-CO2-O2 reforming to syngas in a novel Ba0.5Sr0.5Co0.8Fe0.2O 3-δ oxygen-permeable membrane reactor using LiLaNiO/γ-Al2O3 as catalyst was successfully reported. Excellent reaction performance was achieved with around 92% methane conversion efficiency, 95% CO2 conversion rate, and nearly 8.5mL/min.cm2 oxygen permeation flux. In contrast to the oxygen permeation model with the presence of large concentration of CO2 (under such condition the oxygen permeation flux deteriorates with time), the oxygen permeation flux is really stable under the CH4-CO2-O2 reforming condition.",

keywords = "Ceramic membrane reactor, Methane, Oxygen permeation, Syngas",

author = "Shao, {Zong Ping} and Hui Dong and Xiong, {Guo Xing} and Yang, {Wei Shen}",

year = "2000",

month = jul,

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volume = "11",

pages = "631--634",

journal = "Chinese Chemical Letters",

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TY - JOUR

T1 - Syngas Production Using an Oxygen-Permeating Membrane Reactor with Cofeed of Methane and Carbon Dioxide

AU - Shao, Zong Ping

AU - Dong, Hui

AU - Xiong, Guo Xing

AU - Yang, Wei Shen

PY - 2000/7

Y1 - 2000/7

N2 - CH4-CO2-O2 reforming to syngas in a novel Ba0.5Sr0.5Co0.8Fe0.2O 3-δ oxygen-permeable membrane reactor using LiLaNiO/γ-Al2O3 as catalyst was successfully reported. Excellent reaction performance was achieved with around 92% methane conversion efficiency, 95% CO2 conversion rate, and nearly 8.5mL/min.cm2 oxygen permeation flux. In contrast to the oxygen permeation model with the presence of large concentration of CO2 (under such condition the oxygen permeation flux deteriorates with time), the oxygen permeation flux is really stable under the CH4-CO2-O2 reforming condition.

AB - CH4-CO2-O2 reforming to syngas in a novel Ba0.5Sr0.5Co0.8Fe0.2O 3-δ oxygen-permeable membrane reactor using LiLaNiO/γ-Al2O3 as catalyst was successfully reported. Excellent reaction performance was achieved with around 92% methane conversion efficiency, 95% CO2 conversion rate, and nearly 8.5mL/min.cm2 oxygen permeation flux. In contrast to the oxygen permeation model with the presence of large concentration of CO2 (under such condition the oxygen permeation flux deteriorates with time), the oxygen permeation flux is really stable under the CH4-CO2-O2 reforming condition.

KW - Ceramic membrane reactor

KW - Methane

KW - Oxygen permeation

KW - Syngas

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M3 - 文章

AN - SCOPUS:0345757139

SN - 1001-8417

VL - 11

SP - 631

EP - 634

JO - Chinese Chemical Letters

JF - Chinese Chemical Letters

IS - 7

ER -

Syngas Production Using an Oxygen-Permeating Membrane Reactor with Cofeed of Methane and Carbon Dioxide

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Keywords

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