The Mutual Conversion of CO2 and CO in Dielectric Barrier Discharge (DBD)

Guangyun Zheng; Jiemin Jiang; Yuping Wu; Renxi Zhang; Huiqi Hou

doi:10.1023/A:1022464702294

The Mutual Conversion of CO₂ and CO in Dielectric Barrier Discharge (DBD)

Guangyun Zheng, Jiemin Jiang, Yuping Wu, Renxi Zhang, Huiqi Hou

Fudan University

Research output: Contribution to journal › Article › peer-review

53 Scopus citations

Abstract

Non-equilibrium plasma, which was engendered by dielectric barrier discharge (DBD) was used to analyze the mutual conversion between CO ₂ and CO. The results showed that the conversion ratio of CO increased monotonously with the increasing voltage. But CO₂ was not so. Its conversion ratio reached maximum when the voltage was 3600 V in Ar system. It also showed that the existence of water molecules was more advanageous for the conversion of CO to CO₂ in Ar system than in oxygen system, and the conversion ratio could reach 75.8% when the relative humidity was 100%. We also discussed the energy yield and energy efficiency, and the result was that high voltage and high concentration of reactant was disadvantageous for energy utilization.

Original language	English
Pages (from-to)	59-68
Number of pages	10
Journal	Plasma Chemistry and Plasma Processing
Volume	23
Issue number	1
DOIs	https://doi.org/10.1023/A:1022464702294
State	Published - Mar 2003
Externally published	Yes

Keywords

Carbon dioxide
Carbon monoxide
Conversion ratio
Non-equilibrium plasma

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1023/A:1022464702294

Cite this

@article{2e26af3cb82a4d9faa2157c38bb52d94,

title = "The Mutual Conversion of CO2 and CO in Dielectric Barrier Discharge (DBD)",

abstract = "Non-equilibrium plasma, which was engendered by dielectric barrier discharge (DBD) was used to analyze the mutual conversion between CO 2 and CO. The results showed that the conversion ratio of CO increased monotonously with the increasing voltage. But CO2 was not so. Its conversion ratio reached maximum when the voltage was 3600 V in Ar system. It also showed that the existence of water molecules was more advanageous for the conversion of CO to CO2 in Ar system than in oxygen system, and the conversion ratio could reach 75.8% when the relative humidity was 100%. We also discussed the energy yield and energy efficiency, and the result was that high voltage and high concentration of reactant was disadvantageous for energy utilization.",

keywords = "Carbon dioxide, Carbon monoxide, Conversion ratio, Non-equilibrium plasma",

author = "Guangyun Zheng and Jiemin Jiang and Yuping Wu and Renxi Zhang and Huiqi Hou",

year = "2003",

month = mar,

doi = "10.1023/A:1022464702294",

language = "英语",

volume = "23",

pages = "59--68",

journal = "Plasma Chemistry and Plasma Processing",

issn = "0272-4324",

publisher = "Springer New York",

number = "1",

}

TY - JOUR

T1 - The Mutual Conversion of CO2 and CO in Dielectric Barrier Discharge (DBD)

AU - Zheng, Guangyun

AU - Jiang, Jiemin

AU - Wu, Yuping

AU - Zhang, Renxi

AU - Hou, Huiqi

PY - 2003/3

Y1 - 2003/3

N2 - Non-equilibrium plasma, which was engendered by dielectric barrier discharge (DBD) was used to analyze the mutual conversion between CO 2 and CO. The results showed that the conversion ratio of CO increased monotonously with the increasing voltage. But CO2 was not so. Its conversion ratio reached maximum when the voltage was 3600 V in Ar system. It also showed that the existence of water molecules was more advanageous for the conversion of CO to CO2 in Ar system than in oxygen system, and the conversion ratio could reach 75.8% when the relative humidity was 100%. We also discussed the energy yield and energy efficiency, and the result was that high voltage and high concentration of reactant was disadvantageous for energy utilization.

AB - Non-equilibrium plasma, which was engendered by dielectric barrier discharge (DBD) was used to analyze the mutual conversion between CO 2 and CO. The results showed that the conversion ratio of CO increased monotonously with the increasing voltage. But CO2 was not so. Its conversion ratio reached maximum when the voltage was 3600 V in Ar system. It also showed that the existence of water molecules was more advanageous for the conversion of CO to CO2 in Ar system than in oxygen system, and the conversion ratio could reach 75.8% when the relative humidity was 100%. We also discussed the energy yield and energy efficiency, and the result was that high voltage and high concentration of reactant was disadvantageous for energy utilization.

KW - Carbon dioxide

KW - Carbon monoxide

KW - Conversion ratio

KW - Non-equilibrium plasma

UR - http://www.scopus.com/inward/record.url?scp=0037282252&partnerID=8YFLogxK

U2 - 10.1023/A:1022464702294

DO - 10.1023/A:1022464702294

M3 - 文章

AN - SCOPUS:0037282252

SN - 0272-4324

VL - 23

SP - 59

EP - 68

JO - Plasma Chemistry and Plasma Processing

JF - Plasma Chemistry and Plasma Processing

IS - 1

ER -