Wide-bandgap organic nanocrystals with high mobility and tunable lasing emission

Yin Xiang Li; Wei Liu; Meng Na Yu; Xue Mei Dong; Chang Jin Ou; Mustafa Eginligil; Rui Qing Li; Xin Wen Zhang; Yi Jie Nie; Ling Hai Xie; Chun Xiang Xu; Ju Qing Liu; Wei Huang

doi:10.1039/d0tc05309k

Wide-bandgap organic nanocrystals with high mobility and tunable lasing emission

Yin Xiang Li, Wei Liu, Meng Na Yu, Xue Mei Dong, Chang Jin Ou, Mustafa Eginligil, Rui Qing Li, Xin Wen Zhang, Yi Jie Nie, Ling Hai Xie, Chun Xiang Xu, Ju Qing Liu, Wei Huang

SCHOOL OF FLEXIBLE ELECTRONICS(FUTURE TECHNOLOGIES)|INSTITUTE OF ADVANCED MATERIALS(IAM)

Research output: Contribution to journal › Article › peer-review

11 Scopus citations

Abstract

Here, a wide-bandgap organic nanocrystal is constructed from a steric-functionalized difluorene-based organic semiconductor material 2,2′-bi(9,9′-dimethylfluorene) (BMeF). The synthetic nanocrystal presents superior photoelectric integrated properties, with crystallization-enhanced emission and absolute photoluminescence quantum yield (PLQY) up to 75%, high mobility (0.18 cm²V⁻¹s⁻¹), and low threshold dual-color lasing behavior from ultraviolet (392 nm) to deep-blue (415 nm). Moreover, organic light-emitting diodes (OLEDs) based on BMeF nanocrystals show deep-blue emission with a brightness of 1152 cd m⁻²and turn-on voltage of 2.8 V. This work opens an avenue for high-performance wide-bandgap organic nanocrystals capable of outstanding shortwave emission and high charge mobility.

Original language	English
Pages (from-to)	3171-3176
Number of pages	6
Journal	Journal of Materials Chemistry C
Volume	9
Issue number	9
DOIs	https://doi.org/10.1039/d0tc05309k
State	Published - 7 Mar 2021

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title = "Wide-bandgap organic nanocrystals with high mobility and tunable lasing emission",

abstract = "Here, a wide-bandgap organic nanocrystal is constructed from a steric-functionalized difluorene-based organic semiconductor material 2,2′-bi(9,9′-dimethylfluorene) (BMeF). The synthetic nanocrystal presents superior photoelectric integrated properties, with crystallization-enhanced emission and absolute photoluminescence quantum yield (PLQY) up to 75%, high mobility (0.18 cm2V−1s−1), and low threshold dual-color lasing behavior from ultraviolet (392 nm) to deep-blue (415 nm). Moreover, organic light-emitting diodes (OLEDs) based on BMeF nanocrystals show deep-blue emission with a brightness of 1152 cd m−2and turn-on voltage of 2.8 V. This work opens an avenue for high-performance wide-bandgap organic nanocrystals capable of outstanding shortwave emission and high charge mobility.",

author = "Li, {Yin Xiang} and Wei Liu and Yu, {Meng Na} and Dong, {Xue Mei} and Ou, {Chang Jin} and Mustafa Eginligil and Li, {Rui Qing} and Zhang, {Xin Wen} and Nie, {Yi Jie} and Xie, {Ling Hai} and Xu, {Chun Xiang} and Liu, {Ju Qing} and Wei Huang",

note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry 2021.",

year = "2021",

month = mar,

day = "7",

doi = "10.1039/d0tc05309k",

language = "英语",

volume = "9",

pages = "3171--3176",

journal = "Journal of Materials Chemistry C",

issn = "2050-7526",

publisher = "Royal Society of Chemistry",

number = "9",

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TY - JOUR

T1 - Wide-bandgap organic nanocrystals with high mobility and tunable lasing emission

AU - Li, Yin Xiang

AU - Liu, Wei

AU - Yu, Meng Na

AU - Dong, Xue Mei

AU - Ou, Chang Jin

AU - Eginligil, Mustafa

AU - Li, Rui Qing

AU - Zhang, Xin Wen

AU - Nie, Yi Jie

AU - Xie, Ling Hai

AU - Xu, Chun Xiang

AU - Liu, Ju Qing

AU - Huang, Wei

PY - 2021/3/7

Y1 - 2021/3/7

N2 - Here, a wide-bandgap organic nanocrystal is constructed from a steric-functionalized difluorene-based organic semiconductor material 2,2′-bi(9,9′-dimethylfluorene) (BMeF). The synthetic nanocrystal presents superior photoelectric integrated properties, with crystallization-enhanced emission and absolute photoluminescence quantum yield (PLQY) up to 75%, high mobility (0.18 cm2V−1s−1), and low threshold dual-color lasing behavior from ultraviolet (392 nm) to deep-blue (415 nm). Moreover, organic light-emitting diodes (OLEDs) based on BMeF nanocrystals show deep-blue emission with a brightness of 1152 cd m−2and turn-on voltage of 2.8 V. This work opens an avenue for high-performance wide-bandgap organic nanocrystals capable of outstanding shortwave emission and high charge mobility.

AB - Here, a wide-bandgap organic nanocrystal is constructed from a steric-functionalized difluorene-based organic semiconductor material 2,2′-bi(9,9′-dimethylfluorene) (BMeF). The synthetic nanocrystal presents superior photoelectric integrated properties, with crystallization-enhanced emission and absolute photoluminescence quantum yield (PLQY) up to 75%, high mobility (0.18 cm2V−1s−1), and low threshold dual-color lasing behavior from ultraviolet (392 nm) to deep-blue (415 nm). Moreover, organic light-emitting diodes (OLEDs) based on BMeF nanocrystals show deep-blue emission with a brightness of 1152 cd m−2and turn-on voltage of 2.8 V. This work opens an avenue for high-performance wide-bandgap organic nanocrystals capable of outstanding shortwave emission and high charge mobility.

UR - http://www.scopus.com/inward/record.url?scp=85102373556&partnerID=8YFLogxK

U2 - 10.1039/d0tc05309k

DO - 10.1039/d0tc05309k

M3 - 文章

AN - SCOPUS:85102373556

SN - 2050-7526

VL - 9

SP - 3171

EP - 3176

JO - Journal of Materials Chemistry C

JF - Journal of Materials Chemistry C

IS - 9

ER -

Wide-bandgap organic nanocrystals with high mobility and tunable lasing emission

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