基于过程模拟和随机森林模型的生物质制氢过程因素分析与预测

Li Liu, Peng Jiang, Wei Wang, Tonghuan Zhang, Liwen Mu, Xiaohua Lu, Jiahua Zhu

科研成果: 期刊稿件文章同行评审

3 引用 (Scopus)

摘要

Biomass can replace fossil fuels, reduce greenhouse gas emissions, and is a promising renewable energy source. Co-production of multiple-products has been demonstrated efficient and economically viable process. The techno-economic feasibility of biomass conversion into hydrogen (H2) and activated carbon (AC) route has also been analyzed. However, the selection of raw materials and process parameters become the main barrier for scale-up production. The different types of biomass species and the process conditions affect the yield and quality of the products. In this paper, a process model was developed to simulate the biomass conversion process. H2was produced from biomass through pyrolysis and chemical looping gasification processes. AC was fabricated from biomass through carbonization and activation processes. Then, machine learning was used to build a high-quality prediction model and accordingly explore the importance factors in producing demanded products. The results indicated that process parameters had greater influence than the raw materials on H2 concentration and yield. For example, hydrogen concentration was more relevant (61%) to the reforming temperature, hydrogen concentration in syngas and steam usage, hydrogen yield was more relevant (63%) to the dosage of activation agent and steam usage. Partial dependence plot (PDP) analysis provided the optimal range of processing parameters for maximized production of target products.

投稿的翻译标题Coupling process simulation and random forest model for analyzing and predicting biomass-to-hydrogen conversion
源语言繁体中文
页(从-至)5230-5239
页数10
期刊Huagong Xuebao/CIESC Journal
73
11
DOI
出版状态已出版 - 5 11月 2022

关键词

  • activated carbon
  • biomass
  • hydrogen
  • prediction
  • process simulation
  • random forest

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