A stable singlet biradicaloid siladicarbene: (L:)2Si

Kartik Chandra Mondal, Herbert W. Roesky, Martin C. Schwarzer, Gernot Frenking, Benedikt Niepötter, Hilke Wolf, Regine Herbst-Irmer, Dietmar Stalke

科研成果: 期刊稿件文章同行评审

237 引用 (Scopus)

摘要

A trapped silicon atom: The compound (L:)2Si with low-valent silicon was synthesized from its dichloride biradical precursor (L:) 2SiCl2 by reduction with KC8. Theoretical analysis suggest that there are two donor-acceptor σ bonds L:→Si←:L. There is one σ lone-pair orbital at Si and one π orbital which features significant π-back-donation L:←Si→:L giving short Si-C bonds.

源语言英语
页(从-至)2963-2967
页数5
期刊Angewandte Chemie - International Edition
52
10
DOI
出版状态已出版 - 4 3月 2013
已对外发布

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