Generation and Characterization of the C3O2 Anion with an Unexpected Unsymmetrical Structure

Lina Wang, Sudip Pan, Bo Lu, Xuelin Dong, Hongmin Li, Guohai Deng, Xiaoqing Zeng, Mingfei Zhou, Gernot Frenking

科研成果: 期刊稿件文章同行评审

13 引用 (Scopus)

摘要

The carbon suboxide anion C3O2 is generated in solid neon matrix. It is characterized by infrared absorption spectroscopy as well as quantum chemical calculations to have a planar Cs structure where two CO groups with significantly different bond lengths and angles are attached in a zigzag fashion to the central carbon atom. Bonding analysis indicates that it is best described by the bonding interactions between a neutral CO in a triplet excited state and a doublet excited state of CCO.

源语言英语
页(从-至)4518-4523
页数6
期刊Angewandte Chemie - International Edition
60
9
DOI
出版状态已出版 - 23 2月 2021

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