Generation of stereodefined (Z)-3,4-dihydronaphthalen-1(2H)-ones via copper-catalyzed annulation-cyanotrifluoromethylation of 1,7-enynes

Wen Zhe Ji, Hao Nan Shi, Wen Juan Hao, Ping Wei, Shu Jiang Tu, Bo Jiang

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摘要

A new three-component strategy for the copper-catalyzed annulation–cyanotrifluoromethylation of easily available 1,7-enynes with Togni's reagent and TMSCN is developed. The reaction proceeds smoothly under mild conditions, providing a rapid and concise access to a wide range of stereodefined (Z)-3,4-dihydronaphthalen-1(2H)-ones with a quaternary carbon center in generally good yields. The protocol enjoys wide substrate scope regarding 1,7-enynes, high functional group tolerance and complete stereoselectivity.

源语言英语
文章编号152722
期刊Tetrahedron Letters
64
DOI
出版状态已出版 - 2 2月 2021

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