Low-valent Ge2 and Ge4 species trapped by N-Heterocyclic gallylene

Adinarayana Doddi, Christian Gemel, Manuela Winter, Roland A. Fischer, Catharina Goedecke, Henry S. Rzepa, Gernot Frenking

科研成果: 期刊稿件文章同行评审

46 引用 (Scopus)

摘要

Much π and no ω: Quantum chemical calculations showed that the Ge atoms of the Ga2Ge2 core in Ge2[Ga(DPP)] 2 are not bonded by ω interactions, but rather by a transannular π interaction (see picture). The compound is formed by reduction of (PCy3)·GeCl2 with Ga(DDP)/KC8 which also yielded a further product Ge4[Ga-(DPP)]2 with a Ge2 tetrahedron (DDP=HC(CMeNC6H3-2,6-iPr 2)2).

源语言英语
页(从-至)450-454
页数5
期刊Angewandte Chemie - International Edition
52
1
DOI
出版状态已出版 - 2 1月 2013
已对外发布

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