TY - JOUR
T1 - Recent progress of carbon-based electrocatalytic materials in Lithium-based batteries
AU - Wang, Pengfei
AU - Zhang, Jiahong
AU - Peng, Ying
AU - Hu, Xiulan
AU - Miao, Lei
AU - Ishizaki, Takahiro
N1 - Publisher Copyright:
© 2022 Elsevier B.V.
PY - 2022/7
Y1 - 2022/7
N2 - Lithium‑oxygen, −air, -CO2 are three typical types of Lithium-based batteries, which offer a promising, sustainable, and environment-friendly solution to construct carbon neutral society. Carbon-based cathodes provide active sites for mass and electronic transfer among Li, Li+, O2, Li2O2, LiO2. The synthesis methods of carbon cathode can affect the performance of Lithium-based battery. This review summarizes the fundamentals of carbon-based oxygen evolution reaction (OER) and oxygen reduced reaction (ORR) electrocatalytic reactions, and then explore a few key concerns on the interrelation between synthesis methods and electrocatalytic activities. Then, the most important tactics: defect engineering, heteroatom doping, and structure optimization for enhancement of electrocatalytic activity are presented. Finally, the most recent advances of carbon-based materials from dimensional views are also discussed. The review would provide insightful opportunities as well as the current challenges to accelerate the research and application on carbon-based materials for Lithium-based batteries.
AB - Lithium‑oxygen, −air, -CO2 are three typical types of Lithium-based batteries, which offer a promising, sustainable, and environment-friendly solution to construct carbon neutral society. Carbon-based cathodes provide active sites for mass and electronic transfer among Li, Li+, O2, Li2O2, LiO2. The synthesis methods of carbon cathode can affect the performance of Lithium-based battery. This review summarizes the fundamentals of carbon-based oxygen evolution reaction (OER) and oxygen reduced reaction (ORR) electrocatalytic reactions, and then explore a few key concerns on the interrelation between synthesis methods and electrocatalytic activities. Then, the most important tactics: defect engineering, heteroatom doping, and structure optimization for enhancement of electrocatalytic activity are presented. Finally, the most recent advances of carbon-based materials from dimensional views are also discussed. The review would provide insightful opportunities as well as the current challenges to accelerate the research and application on carbon-based materials for Lithium-based batteries.
KW - Carbon materials
KW - Electrocatalysts
KW - Lithium-based batteries
KW - OER/ORR
UR - http://www.scopus.com/inward/record.url?scp=85123121328&partnerID=8YFLogxK
U2 - 10.1016/j.susmat.2021.e00384
DO - 10.1016/j.susmat.2021.e00384
M3 - 文献综述
AN - SCOPUS:85123121328
SN - 2214-9937
VL - 32
JO - Sustainable Materials and Technologies
JF - Sustainable Materials and Technologies
M1 - e00384
ER -
