Towards Fast Bayesian inference of equivalent circuit parameters of perovskite solar cell

Jian Sun, Jintian Pan, Qing Song, Yang Liu, Yue Wang, Yonghua Chen, Deli Li

Research output: Contribution to journalArticlepeer-review

Abstract

Interpreting current–voltage data through an equivalent circuit model offers a rapid, real-time method for analyzing the internal changes in perovskite solar cells. Recent studies have utilized Bayesian inference to solve this inverse problem, but the inference time remains a bottleneck for practical applications. In this work, we propose a modified approach that simplifies the likelihood function within the Bayesian inference process. By leveraging the inherent characteristics of the equivalent circuit, we reduce the five-parameter model to a more efficient three-parameter approximation, greatly enhancing parameter estimation efficiency. Our results demonstrate that the simplified model retains the same level of computational accuracy. In addition, it reduces inference time by a factor of over 15, from hundreds of seconds to just a few seconds on Google Colaboratory using a CPU with two Xeon cores (2.2 GHz). The number of inference steps also decreases from tens of thousands to only a few hundred. This significant improvement accelerates the overall inference process, enabling faster, real-time monitoring and aging analysis of perovskite solar cells. Our method offers an intelligent solution for efficiently analyzing solar cell performance through Bayesian inference, advancing both research and engineering applications.

Original languageEnglish
Article number113308
JournalSolar Energy
Volume288
DOIs
StatePublished - 1 Mar 2025

Keywords

  • Bayesian inference
  • Equivalent circuit model
  • Metal halide perovskite
  • Solar cell

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