TY - JOUR
T1 - Investigation of Mass Transfer Characteristics of SO2Absorption into NaOH in a Multichannel Ceramic Membrane Contactor
AU - Kong, Xiangli
AU - Gong, Dawei
AU - Ke, Wei
AU - Qiu, Minghui
AU - Fu, Kaiyun
AU - Xu, Peng
AU - Chen, Xianfu
AU - Fan, Yiqun
N1 - Publisher Copyright:
Copyright © 2020 American Chemical Society.
PY - 2020/6/10
Y1 - 2020/6/10
N2 - A ceramic membrane with multichannels generally has a higher specific area and larger throughput compared to that with a single channel, which is beneficial to the industrialization of ceramic membrane contactors for SO2 absorption. In this work, the mass transfer performance of SO2 absorption into NaOH solution was investigated at various gas and liquid operating conditions in a membrane contactor packed with a 19-channel hydrophilic membrane. The results showed that increasing the NaOH concentration can offset the effect of membrane thickness. To analyze the mass transfer process, a 3D mass transfer model was developed to simulate the concentration distribution of the components. The simulated SO2 fluxes were consistent with the experimental results. Additionally, the mass transfer model was applied to optimize the structure of channels in multichannel ceramic membranes. The operational mode of the multichannel ceramic membrane is optimized by blocking some inside channels to reduce the mass transfer resistance.
AB - A ceramic membrane with multichannels generally has a higher specific area and larger throughput compared to that with a single channel, which is beneficial to the industrialization of ceramic membrane contactors for SO2 absorption. In this work, the mass transfer performance of SO2 absorption into NaOH solution was investigated at various gas and liquid operating conditions in a membrane contactor packed with a 19-channel hydrophilic membrane. The results showed that increasing the NaOH concentration can offset the effect of membrane thickness. To analyze the mass transfer process, a 3D mass transfer model was developed to simulate the concentration distribution of the components. The simulated SO2 fluxes were consistent with the experimental results. Additionally, the mass transfer model was applied to optimize the structure of channels in multichannel ceramic membranes. The operational mode of the multichannel ceramic membrane is optimized by blocking some inside channels to reduce the mass transfer resistance.
UR - http://www.scopus.com/inward/record.url?scp=85088905315&partnerID=8YFLogxK
U2 - 10.1021/acs.iecr.0c01327
DO - 10.1021/acs.iecr.0c01327
M3 - 文章
AN - SCOPUS:85088905315
SN - 0888-5885
VL - 59
SP - 11054
EP - 11062
JO - Industrial and Engineering Chemistry Research
JF - Industrial and Engineering Chemistry Research
IS - 23
ER -