TY - JOUR
T1 - Investigation on strengthening effect of metal foams in enlarged microchannels for heterogeneous liquid-liquid mass transfer
AU - Shen, Zhaoyang
AU - Wang, Qichao
AU - Xu, Feng
AU - Zhou, Xiang
AU - Ni, Lei
AU - Cheng, Zhiquan
AU - Jiang, Juncheng
N1 - Publisher Copyright:
© 2025
PY - 2025/9
Y1 - 2025/9
N2 - In this work, to enhance the mass transfer process between two heterogeneous phases in the enlarged microchannel, the metal foam was filled into the quartz channel. First, the homogeneous iodate system was employed to investigate the mixing efficiency of fluids flowing through the metal foam. The results indicate that the mixing efficiency improves with increasing metal foam length and pore density. Secondly, the extraction and mass transfer efficiency of metal foam was studied by using the n-butanol-succinic acid system (heterogeneous). The results showed that the extraction efficiency and mass transfer performance of metal foam with a pore density of 60 PPI and a length of 10 cm were the best, reaching 56 % and 0.297 s-1. Finally, the enhancement of metal foam on the reaction process was investigated by the oxidation process of phenylene sulfide, and the metal foam with the best mass transfer performance was selected for the experiment. Under the residence time of 15 min, the conversion of the raw material reached 86.57 %, which was nearly 4 times higher than that channel without structural inserts. Therefore, it is a very meaningful strategy to strengthen the mass transfer process by using the enlarged microchannels filled with metal foam.
AB - In this work, to enhance the mass transfer process between two heterogeneous phases in the enlarged microchannel, the metal foam was filled into the quartz channel. First, the homogeneous iodate system was employed to investigate the mixing efficiency of fluids flowing through the metal foam. The results indicate that the mixing efficiency improves with increasing metal foam length and pore density. Secondly, the extraction and mass transfer efficiency of metal foam was studied by using the n-butanol-succinic acid system (heterogeneous). The results showed that the extraction efficiency and mass transfer performance of metal foam with a pore density of 60 PPI and a length of 10 cm were the best, reaching 56 % and 0.297 s-1. Finally, the enhancement of metal foam on the reaction process was investigated by the oxidation process of phenylene sulfide, and the metal foam with the best mass transfer performance was selected for the experiment. Under the residence time of 15 min, the conversion of the raw material reached 86.57 %, which was nearly 4 times higher than that channel without structural inserts. Therefore, it is a very meaningful strategy to strengthen the mass transfer process by using the enlarged microchannels filled with metal foam.
KW - Extraction efficiency
KW - Mass transfer
KW - Metal foam
KW - Microreactor
KW - Mixing efficiency
UR - http://www.scopus.com/inward/record.url?scp=105007030410&partnerID=8YFLogxK
U2 - 10.1016/j.cep.2025.110379
DO - 10.1016/j.cep.2025.110379
M3 - 文章
AN - SCOPUS:105007030410
SN - 0255-2701
VL - 215
JO - Chemical Engineering and Processing - Process Intensification
JF - Chemical Engineering and Processing - Process Intensification
M1 - 110379
ER -