Copper-catalyzed three-component annulation toward pyrroles via the cleavage of two C-C bonds in 1,3-dicarbonyls

Gaochen Xu; Luchao Li; Binyan Xu; Zheng Fang; Jindian Duan; Kai Guo

doi:10.1039/d3cc02681g

Copper-catalyzed three-component annulation toward pyrroles via the cleavage of two C-C bonds in 1,3-dicarbonyls

Gaochen Xu, Luchao Li, Binyan Xu, Zheng Fang, Jindian Duan, Kai Guo

生物与制药工程学院

Nanjing Tech University

科研成果: 期刊稿件 › 文章 › 同行评审

9 引用（Scopus）

摘要

The first copper-catalyzed three-component annulation of α,β-unsaturated ketoximes, 1,3-dicarbonyls and paraformaldehyde has been documented. This novel strategy achieved the two C-C bond cleavage of 1,3-dicarbonyl compounds directly as a single-carbon synthon and provided a new and highly efficient method for the synthesis of 2,3-disubstituted pyrroles in moderate to good yields with broad functional group compatibility.

源语言	英语
页（从-至）	10636-10639
页数	4
期刊	Chemical Communications
卷	59
期	71
DOI	https://doi.org/10.1039/d3cc02681g
出版状态	已出版 - 9 8月 2023

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abstract = "The first copper-catalyzed three-component annulation of α,β-unsaturated ketoximes, 1,3-dicarbonyls and paraformaldehyde has been documented. This novel strategy achieved the two C-C bond cleavage of 1,3-dicarbonyl compounds directly as a single-carbon synthon and provided a new and highly efficient method for the synthesis of 2,3-disubstituted pyrroles in moderate to good yields with broad functional group compatibility.",

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T1 - Copper-catalyzed three-component annulation toward pyrroles via the cleavage of two C-C bonds in 1,3-dicarbonyls

AU - Xu, Gaochen

AU - Li, Luchao

AU - Xu, Binyan

AU - Fang, Zheng

AU - Duan, Jindian

AU - Guo, Kai

PY - 2023/8/9

Y1 - 2023/8/9

N2 - The first copper-catalyzed three-component annulation of α,β-unsaturated ketoximes, 1,3-dicarbonyls and paraformaldehyde has been documented. This novel strategy achieved the two C-C bond cleavage of 1,3-dicarbonyl compounds directly as a single-carbon synthon and provided a new and highly efficient method for the synthesis of 2,3-disubstituted pyrroles in moderate to good yields with broad functional group compatibility.

AB - The first copper-catalyzed three-component annulation of α,β-unsaturated ketoximes, 1,3-dicarbonyls and paraformaldehyde has been documented. This novel strategy achieved the two C-C bond cleavage of 1,3-dicarbonyl compounds directly as a single-carbon synthon and provided a new and highly efficient method for the synthesis of 2,3-disubstituted pyrroles in moderate to good yields with broad functional group compatibility.

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U2 - 10.1039/d3cc02681g

DO - 10.1039/d3cc02681g

M3 - 文章

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AN - SCOPUS:85169292273

SN - 1359-7345

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SP - 10636

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JO - Chemical Communications

JF - Chemical Communications

IS - 71

ER -

Copper-catalyzed three-component annulation toward pyrroles via the cleavage of two C-C bonds in 1,3-dicarbonyls

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