Visible light mediated regioselective 1,3-oxylallylation of aryl cyclopropanes under redox-neutral conditions

Ding Xing Wang; Hui Wang; Yao Xu; Chi Zhang; Chao Feng

doi:10.1039/d3qo00281k

Visible light mediated regioselective 1,3-oxylallylation of aryl cyclopropanes under redox-neutral conditions

Ding Xing Wang, Hui Wang, Yao Xu, Chi Zhang, Chao Feng

化学与分子工程学院

Nanjing Tech University

科研成果: 期刊稿件 › 文章 › 同行评审

6 引用（Scopus）

摘要

A photoredox catalysed 1,3-oxylallylation of aryl cyclopropanes was accomplished by reaction with carboxylic acids and allyl sulfones. The redox-neutral reaction proceeded in a highly regioselective manner under mild conditions with good functional group compatibility. Simple operation and successful application to the late-stage functionalization of several natural product and pharmaceutical molecule related carboxylic acids add extra merits to the current protocol.

源语言	英语
页（从-至）	2147-2154
页数	8
期刊	Organic Chemistry Frontiers
卷	10
期	9
DOI	https://doi.org/10.1039/d3qo00281k
出版状态	已出版 - 1 4月 2023

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10.1039/d3qo00281k

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abstract = "A photoredox catalysed 1,3-oxylallylation of aryl cyclopropanes was accomplished by reaction with carboxylic acids and allyl sulfones. The redox-neutral reaction proceeded in a highly regioselective manner under mild conditions with good functional group compatibility. Simple operation and successful application to the late-stage functionalization of several natural product and pharmaceutical molecule related carboxylic acids add extra merits to the current protocol.",

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AU - Wang, Ding Xing

AU - Wang, Hui

AU - Xu, Yao

AU - Zhang, Chi

AU - Feng, Chao

PY - 2023/4/1

Y1 - 2023/4/1

N2 - A photoredox catalysed 1,3-oxylallylation of aryl cyclopropanes was accomplished by reaction with carboxylic acids and allyl sulfones. The redox-neutral reaction proceeded in a highly regioselective manner under mild conditions with good functional group compatibility. Simple operation and successful application to the late-stage functionalization of several natural product and pharmaceutical molecule related carboxylic acids add extra merits to the current protocol.

AB - A photoredox catalysed 1,3-oxylallylation of aryl cyclopropanes was accomplished by reaction with carboxylic acids and allyl sulfones. The redox-neutral reaction proceeded in a highly regioselective manner under mild conditions with good functional group compatibility. Simple operation and successful application to the late-stage functionalization of several natural product and pharmaceutical molecule related carboxylic acids add extra merits to the current protocol.

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DO - 10.1039/d3qo00281k

M3 - 文章

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SN - 2052-4110

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JO - Organic Chemistry Frontiers

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ER -

Visible light mediated regioselective 1,3-oxylallylation of aryl cyclopropanes under redox-neutral conditions

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