Palladium-catalyzed alkenyl C-H bond sulfonylation reaction using organosulfonyl chlorides

Yun He Xu; Min Wang; Ping Lu; Teck Peng Loh

doi:10.1016/j.tet.2013.01.071

Palladium-catalyzed alkenyl C-H bond sulfonylation reaction using organosulfonyl chlorides

Yun He Xu, Min Wang, Ping Lu, Teck Peng Loh

科研成果: 期刊稿件 › 文章 › 同行评审

41 引用（Scopus）

摘要

A Pd-catalyzed alkenyl C-H bond direct sulfonylation of vinyl pyridine and enamides was developed. Various arylsulfonyl chlorides were tested in this reaction and the desired products were obtained in good yields. Moreover, the alkyl sulfonyl chloride could also be used though the yield was lower. A possible Pd(II)/Pd(IV) catalytic pathway involved in this coupling reaction was proposed.

源语言	英语
页（从-至）	4403-4407
页数	5
期刊	Tetrahedron
卷	69
期	22
DOI	https://doi.org/10.1016/j.tet.2013.01.071
出版状态	已出版 - 3 6月 2013
已对外发布	是

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abstract = "A Pd-catalyzed alkenyl C-H bond direct sulfonylation of vinyl pyridine and enamides was developed. Various arylsulfonyl chlorides were tested in this reaction and the desired products were obtained in good yields. Moreover, the alkyl sulfonyl chloride could also be used though the yield was lower. A possible Pd(II)/Pd(IV) catalytic pathway involved in this coupling reaction was proposed.",

keywords = "Coupling, Enamide, Palladium, Sulfonylation, Vinyl pyridine",

author = "Xu, {Yun He} and Min Wang and Ping Lu and Loh, {Teck Peng}",

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T1 - Palladium-catalyzed alkenyl C-H bond sulfonylation reaction using organosulfonyl chlorides

AU - Xu, Yun He

AU - Wang, Min

AU - Lu, Ping

AU - Loh, Teck Peng

PY - 2013/6/3

Y1 - 2013/6/3

N2 - A Pd-catalyzed alkenyl C-H bond direct sulfonylation of vinyl pyridine and enamides was developed. Various arylsulfonyl chlorides were tested in this reaction and the desired products were obtained in good yields. Moreover, the alkyl sulfonyl chloride could also be used though the yield was lower. A possible Pd(II)/Pd(IV) catalytic pathway involved in this coupling reaction was proposed.

AB - A Pd-catalyzed alkenyl C-H bond direct sulfonylation of vinyl pyridine and enamides was developed. Various arylsulfonyl chlorides were tested in this reaction and the desired products were obtained in good yields. Moreover, the alkyl sulfonyl chloride could also be used though the yield was lower. A possible Pd(II)/Pd(IV) catalytic pathway involved in this coupling reaction was proposed.

KW - Coupling

KW - Enamide

KW - Palladium

KW - Sulfonylation

KW - Vinyl pyridine

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DO - 10.1016/j.tet.2013.01.071

M3 - 文章

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SN - 0040-4020

VL - 69

SP - 4403

EP - 4407

JO - Tetrahedron

JF - Tetrahedron

IS - 22

ER -

Palladium-catalyzed alkenyl C-H bond sulfonylation reaction using organosulfonyl chlorides

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